The phase 4 world of thrillers by various artists.  Decca ZAL10616P SPA160, published in 1969.

Record contains versions of :

Theme from 2001, Spellbound, I Spy, Route 66, Windmills of your mind(Thomas Crown Affair), The man with the Golden Arm, The Avengers, North by Northwest, Charade, The Saint, On the waterfront.